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dc.contributor.authorPousaneh, Faezeh
dc.contributor.authorde Wijn, Astrid S.
dc.date.accessioned2021-01-20T10:55:07Z
dc.date.available2021-01-20T10:55:07Z
dc.date.created2021-01-18T18:41:22Z
dc.date.issued2020
dc.identifier.issn0031-9007
dc.identifier.urihttps://hdl.handle.net/11250/2723876
dc.description.abstractTransport properties of dense fluids are fundamentally challenging, because the powerful approaches of equilibrium statistical physics cannot be applied. Polar fluids compound this problem, because the long-range interactions preclude the use of a simple effective diameter approach based solely on hard spheres. Here, we develop a kinetic theory for dipolar hard-sphere fluids that is valid up to high density. We derive a mathematical approximation for the radial distribution function at contact directly from the equation of state, and use it to obtain the shear viscosity. We also perform molecular-dynamics simulations of this system and extract the shear viscosity numerically. The theoretical results compare favorably to the simulations.en_US
dc.language.isoengen_US
dc.publisherAmerican Physical Societyen_US
dc.titleKinetic Theory and Shear Viscosity of Dense Dipolar Hard Sphere Liquidsen_US
dc.typePeer revieweden_US
dc.typeJournal articleen_US
dc.description.versionpublishedVersionen_US
dc.source.journalPhysical Review Lettersen_US
dc.identifier.doi10.1103/PhysRevLett.124.218004
dc.identifier.cristin1873668
dc.description.localcode© American Physical Society 2020.en_US
cristin.ispublishedtrue
cristin.fulltextpreprint
cristin.qualitycode2


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