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dc.contributor.authorAarnæs, Trygve Storm
dc.contributor.authorRingdalen, Eli
dc.contributor.authorTangstad, Merete
dc.date.accessioned2021-01-08T08:22:29Z
dc.date.available2021-01-08T08:22:29Z
dc.date.created2021-01-07T15:26:06Z
dc.date.issued2020
dc.identifier.issn2045-2322
dc.identifier.urihttps://hdl.handle.net/11250/2722119
dc.description.abstractSilicon carbide (SiC) formation plays an important role during the production of elemental silicon. SiC forms through a high temperature reaction between silicon monoxide gas (SiO) and carbon. Currently, the carbon sources are solids, however fnding a way of substituting the solid carbon with methane could have several advantages. SiC formation was studied in argon, hydrogen and methane containing atmospheres at 1650 °C and 1750 °C. SiO gas was generated from pellets of a 1:2 molar ratio of SiC and silica (SiO2). The reactions were investigated through CO of-gas analysis in conjunction with measuring the weight change. After each experiment, the reaction products were examined in a scanning electron microscope with secondary electrons and through energy-dispersive X-ray spectroscopy. It was confrmed that SiC may form from SiO and methane. Increasing the methane content to 5% caused a signifcant increase in SiC formation. Furthermore, the SiC structure was also highly sensitive to the methane content that was used. In addition, the SiO producing reaction was afected by hydrogen. The hydrogen lead to an increased rate of SiO formation relative to what was seen in argon. The efect of hydrogen was most pronounced at 1750 °C which is right after the melting of silica.en_US
dc.language.isoengen_US
dc.publisherNature Researchen_US
dc.rightsNavngivelse 4.0 Internasjonal*
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/deed.no*
dc.titleSilicon carbide formation from methane and silicon monoxideen_US
dc.typePeer revieweden_US
dc.typeJournal articleen_US
dc.description.versionpublishedVersionen_US
dc.source.volume10en_US
dc.source.journalScientific Reportsen_US
dc.source.issue1en_US
dc.identifier.doi10.1038/s41598-020-79006-6
dc.identifier.cristin1867240
dc.description.localcode© The Author(s) 2020. This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.en_US
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