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On Mathematical Modeling and Numerical Simulation of Chemical Kinetics in Turbulent Lean Premixed Combustion

Lilleberg, Bjørn
Doctoral thesis
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491949_FULLTEXT01.pdf (Locked)
URI
http://hdl.handle.net/11250/234564
Date
2011
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  • Institutt for energi og prosessteknikk [4512]
Abstract
This thesis investigates turbulent reacting lean premixed flows with detailed treatment of the chemistry. First, the fundamental equations which govern laminar and turbulent reacting flows are presented.

A perfectly stirred reactor numerical code is developed to investigate the role of unmixedness and chemical kinetics in driving combustion instabilities. This includes both global single-step and detailed chemical kinetic mechanisms. The single-step mechanisms predict to some degree a similar behavior as the detailed mechanisms. However, it is shown that simple mechanisms can by themselves introduce instabilities.

Magnussen’s Eddy Dissipation Concept (EDC) for turbulent combustion is implemented in the open source CFD toolbox OpenFOAM R for treatment of both fast and detailed chemistry. RANS turbulence models account for the turbulent compressible flow.

A database of pre-calculated chemical time scales, which contains the influence of chemical kinetics, is coupled to EDC with fast chemistry to account for local extinction in both diffusion and premixed flames. Results are compared to fast and detailed chemistry calculations. The inclusion of the database shows significantly better results than the fast chemistry calculations while having a comparably small computational cost.

Numerical simulations of four piloted lean premixed jet flames falling into the "well stirred reactor/broken reaction zones" regime, with strong finite-rate chemistry effects, are performed. Measured and predicted scalars compare well for the two jets with the lowest velocities. The two jets with the highest velocities experience extinction and reignition, and the simulations are able to capture the decrease and increase of the OH mass fractions, but the peak values are higher than in the experiments.

Also numerical simulations of a lean premixed lifted jet flame with high sensitivity to turbulence modeling and chemical kinetics are performed. Limitations of the applied turbulence and chemical kinetics models are demonstrated and discussed.
Publisher
Norges teknisk-naturvitenskapelige universitet, Fakultet for ingeniørvitenskap og teknologi, Institutt for energi- og prosessteknikk
Series
Doktoravhandlinger ved NTNU, 1503-8181; 2011:206

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