Blar i NTNU Open på forfatter "Mæhlen, Jan Petter"
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A Method for Controlled Oxide and Carbon Coating of Silicon Nanoparticles as Anode in Lithium-Ion Batteries
Orderud Skare, Marte (Master thesis, 2017)Silicon has emerged as a promising alternative to graphite in lithium-ion batteries. Silicon can, theoretically, provide up to ten times higher capacity due to its high alloying capabilities with lithium. This improvement ... -
A Stability Study of Substoichiometric Silicon Nitride Nanoparticles as Active Anode Material for Li-ion Batteries
Krogsæter, Henrik (Master thesis, 2019)De fremragende elektrokjemiske egenskapene til understøkiometrisk silisium nitrid (SiNx) har gjort dette material til en potensiell kandidat for neste generasjons Li-ion batteri aktive anode materiale. Den først litsieringen ... -
Anodes for Li‑ion batteries prepared from microcrystalline silicon and enabled by binder’s chemistry and pseudo‑self‑healing
Foss, Carl Erik Lie; Stephan, Müssig; Svensson, Ann Mari; Vie, Preben Joakim Svela; Ulvestad, Asbjørn; Mæhlen, Jan Petter; Koposov, Alexey (Peer reviewed; Journal article, 2020)Silicon, while suffering from major degradation issues, has been recognized as a next promising material to replace currently used graphite in the anodes of Li-ion batteries. Several pathways to mitigate the capacity fading ... -
Carbon-Coated Industrial-Grade Silicon as Potential Anode Material in Lithium-Ion Batteries
Backer, Lasse August Dørum (Master thesis, 2021)Silisium (Si) er et lovende anodemateriale for neste generasjons litium-ione-batterier (LIB) grunnet dens evne til å reversibelt danne legeringer med høy litiumkonsentrasjon. Dette gir en ekstremt høy gravimetrisk kapasitet ... -
Enabling the use of lithium bis(trifluoromethanesulfonyl)imide as electrolyte salt for Li-ion batteries based on silicon anodes and Li(Ni0.4Co0.4Mn0.2)O2 cathodes by salt additives
Asheim, Karina; Holsen, I.F.; Renmann, V.; Blanco, Maria Valeria; Vullum, Per Erik; Wagner, Nils Peter; Mæhlen, Jan Petter; Svensson, Ann Mari (Journal article; Peer reviewed, 2024)Lithium bis(trifluoromethanesulfonyl)imide (LiFSI) is a promising alternative salt for Li-ion batteries. Unlike the conventional LiPF6, it is not prone to HF formation, and thus resistant to moisture. However, for cell ... -
Improved electrochemical performance and solid electrolyte interphase properties of electrolytes based on lithium bis(fluorosulfonyl)imide for high content silicon anodes
Asheim, Karina; Vullum, Per Erik; Wagner, Nils Peter; Andersen, Hanne Flåten; Mæhlen, Jan Petter; Svensson, Ann Mari (Journal article; Peer reviewed, 2022)Electrodes containing 60 wt% micron-sized silicon were investigated with electrolytes containing carbonate solvents and either LiPF6 or lithium bis(fluorosulfonyl)imide (LiFSI) salt. The electrodes showed improved performance, ... -
Morphology effects in MgH2 anode for lithium ion batteries
El-Kharbachi, Abdelouahab; Andersen, Hanne Flåten; Sørby, Magnus Helgerud; Vullum, Per Erik; Mæhlen, Jan Petter; Hauback, Bjørn (Journal article, 2017)In order to acquire reproducible electrodes relevant for Li ion batteries new MgH2 electrodes are successfully obtained from homogenous slurries in N-Methyl-2-Pyrrolidone “NMP” solvent. The electrodes are aimed to elucidate ... -
On the Cycling Performance and Stability of Silicon-Based Anodes in Lithium-Ion Batteries - Revealing Challenges and Failure Mechanisms Using Post Mortem Analyses
Kaland, Henning (Master thesis, 2017)Li-ion batteries with improved energy density can be obtained by increasing the Si content in the graphite electrode, or replace it entirely with a Si based electrode. This may have the additional benefit of improving ... -
Silicon Nanoparticle Ensembles for Lithium-Ion Batteries Elucidated by Small-Angle Neutron Scattering
Lai, Samson Yuxiu; Knudsen, Kenneth Dahl; Sejersted, Benjamin Tjeltveit; Ulvestad, Asbjørn; Mæhlen, Jan Petter; Koposov, Alexey (Journal article; Peer reviewed, 2019)Silicon in the form of nanoparticles has attracted significant interest in the field of lithium-ion batteries due to the enormous capability of lithium intake. In the present work we demonstrate the characterization of ... -
Silicon-carbon composite anodes from industrial battery grade silicon
Foss, Carl Erik Lie; Andersen, Hanne Flåten; Ulvestad, Asbjørn; Kirkengen, Martin; Vullum, Per Erik; Voje, Jorunn; Tronstad, Ragnar; Mokkelbost, Tommy; Mæhlen, Jan Petter (Journal article; Peer reviewed, 2019)In this work, silicon/carbon composites for anode electrodes of Li-ion batteries are prepared from Elkem’s Silgrain® line. Gentle ball milling is used to reduce particle size of Silgrain, and the resulting Si powder consists ... -
Stoichiometry-Controlled Reversible Lithiation Capacity in Nanostructured Silicon Nitrides Enabled by in Situ Conversion Reaction
Ulvestad, Asbjørn; Skare, Marte Orderud; Foss, Carl Erik Lie; Krogsæter, Henrik; Reichstein, Jakob; Preston, Thomas J.; Mæhlen, Jan Petter; Andersen, Hanne Flåten; Koposov, Alexey (Peer reviewed; Journal article, 2021)In modern Li-based batteries, alloying anode materials have the potential to drastically improve the volumetric and specific energy storage capacity. For the past decade silicon has been viewed as a “Holy Grail” among these ... -
Understanding Capacity Fading of MgH2 Conversion-Type Anodes via Structural Morphology Changes and Electrochemical Impedance
El-Kharbachi, Abdelouahab; Hu, Yang; Sørby, Magnus Helgerud; Vullum, Per Erik; Mæhlen, Jan Petter; Fjellvåg, Helmer; Hauback, Bjørn (Journal article; Peer reviewed, 2018)Previous studies have demonstrated that MgH2 is a promising conversion-type anode toward Li with high capacity (2037 mAh/g) and low discharge/charge overpotential hysteresis. A major challenge is the capacity loss after a ...